Jakob K. Staab

Jan 17, 2025 | dx.doi.org | Toby Thompson |Jakob K. Staab |Nicholas F. Chilton |J. D. Patrick

1. IntroductionClick to copy section linkSection link copied!Knowledge of a chemical system’s Hamiltonian operator is essential for describing both static properties and its evolution through time.

Oct 23, 2024 | pubs.rsc.org | Rizwan Nabi |Benjamin Atkinson |Jakob K. Staab |Jonathan M. Skelton

The impact of low-energy phonon lifetimes on the magnetic relaxation in a dysprosocenium single-molecule magnet Developing molecular spin technologies requires microscopic knowledge of their spin-dynamics. Calculation of phonon modes, phonon scattering and spin-phonon coupling for a dysprosocenium single-molecule magnet (SMM) give simulations of spin-dynamics that agree with experiment.

Apr 26, 2024 | pubs.rsc.org | Jakob K. Staab |Mohammed Rahman |Nicholas F. Chilton

Intramolecular bridging strategies to suppress two-phonon Raman spin relaxation in dysprosocenium single-molecule magnets Dy(III) bis-cyclopentadienyl (Cp) sandwich compounds exhibit extremely strong single-ion magnetic anisotropy which imbues them with magnetic memory and has put them at the forefront of high-performance single-molecule magnets (SMMs).

Jun 28, 2023 | pubs.rsc.org | Andrea Mattioni |Jakob K. Staab |Daniel Reta |Jonathan M. Skelton

Spin–phonon coupling and magnetic relaxation in single-molecule magnets† Jon G. C. Kragskow,a   Andrea Mattioni,*a   Jakob K. Staab, a   Daniel Reta, abcd   Jonathan M. Skelton *a  and  Nicholas F. Chilton *a   Abstract Electron–phonon coupling is important in many physical phenomena, e.g. photosynthesis, catalysis and quantum information processing, but its impacts are difficult to grasp on the microscopic level.

Jun 16, 2023 | dx.doi.org | Jonathan M. Skelton |Nicholas F. Chilton |Barak Alnami |Jakob K. Staab

AbstractAnisotropy in the magnetic susceptibility strongly influences the paramagnetic shifts seen in nuclear magnetic resonance (NMR) and magnetic resonance imaging (MRI) experiments.